Facilities and Key Instruments

Our three home-built cryo-SNOMs has capability of nano-imaging down to resolution of 15nm and temperature of 18K with energy ranging from visible (600nm-1.2um) to MIR (3um-11um) and THz(1-2THz). The systems have extendable, multi-messenger functions such has nano-photocurrent mapping, KPFM and MFM as well.
Spatial resolution 10 nm, scanned area 50×50 μm2, Lasers: mid-IR QCLs & CO2; Difference frequency generation 500-2500 cm-1, pump-probe capabilities.
Articles [305] [310] [319] [323] [327]

Our second of three home-built cryogenic SNOMs primarily focuses on nearfield spectroscopy and imaging in the THz frequency band (0.4-2 THz) with spatial resolution down to 50 nm and with tunable temperature control down to 25 K. The system is capable of THz scattering, ultra-fast optical pump-THz probe, ultra-fast optical pump-THz emission, and 2D THz spectroscopy (under development) measurements, using both a high-field THz source (LNO3) and a low-field rate THz source (PCA), all with nano-scale resolution. Detection of the nano-THz signal occurs in the time-domain using electro-optic sampling techniques that provides both amplitude and phase information. The sample exchange apparatus allows for high-throughput measurements and with in-situ electrical contacts to the sample for electrical gating, current drive, resistivity measurements, and magnetic fields, among a host of other possibilities. Articles [261], [310], [322]

Spectral range: 30-25,000 cm-1. Temperature range: 5-300 K. Magnetic field < 9 T. Microsample capability. Reflectance, transmission, Kerr/Faraday rotation. Bruker Interferometer, Oxford split-coil magnet. Home-built cryogenics and optics. Articles [198][161] [137] [136] [122] [119]

Cryosnom-3 is our third home-built cryogenic SNOM. Cryonom-3 vacuum pressure can reach down to ~ 10^-11 torr and can work at 18 K-350 K. The beam lines and detectors covers the spectral range of 700 nm-116000 nm. At all these wavelengths, the spatial resolution of the scattering light measurement can reach down to 20 nm. Besides the optical measurement capability, side-band KPFM and MFM are also integrated into the system. In addition, there are 9 electrodes on the sample holder, allowing in-situ electrical transport and nano-photocurrent measurements. Check back in the future for links to papers published using Cryo-SNOM-III.

The Attocube cryogenic AFM/MFM is one of our newest instruments. It has a liquid helium-based cryostat with sample temperature variable from 1.8 K to room temperature and magnetic field up to 9T. This cantilever-based atomic force microscope (AFM) with interferometric detection is primarily used for magnetic force microscopy (MFM) to image magnetic domains in bulk, thin film, and device-based samples. With in-situ transport capabilities, this instrument is ideal for investigating magnetic and superconducting phases of materials and devices. Check back in the future for links to papers published using the Attocube cryogenic AFM/MFM.

The broad family of scanning probe techniques accessible with a traditional cantilever-mounted atomic force microscope (AFM) permits simultaneous characterization of topographic (AFM), magnetic (MFM), electro-potential (KPFM), opto-electronic (nano-photocurrent), optical (SNOM, nano-THz, nano-PL), and non-linear optical (nano-SHG) behavior at the nanoscale. This form of multi-messenger nano-imaging provides unprecedented access to the rich interplay of spatially-correlated emergent properties in quantum materials. Articles [281] [294] [300] [302] [314]